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    ●Parsons et al., J. Electroanal. Chem. 1973, 44, 1

    ●Osawa et al., Angewa. Chem., Int. Eds. 2005, 44, 5694, 2010,49,1,

    ●JPCB,2006,110,16559, 11912

    ●Chen et al., Angewa. Chem., Int. Eds. 2006, 45, 981,

    ● Langmuir, 2006, 22, 10399, J. Phys. Chem. B, 2006, 110, 9534.

    ● ChemPhysChem, 2007, 8, 380

    ●Cuesta&Osawa,  ACS Catal. 2012, 2, 728

     

     

    ●Formate adsorption/desorption is just an individual process which occurs in parallel with HCOOH oxidation.

    ●HCOOad limits the surface sites for HCOOH oxidation.

    ●Phys. Chem. Chem. Phys., 2013, 15 (12), 4367

     

    ●Chen et al., 2006. Bridge-bonded formate: Active intermediate or spectator species in formic acid oxidation on a Pt film electrode Langmuir 22: 10399-408.

    ●Osawa et al., 2011. The Role of Bridge-Bonded Adsorbed Formate in the Electrocatalytic Oxidation of Formic Acid on Platinum Angewandte Chemie-International Edition 50: 1159-63.

     

    ●在1D Pt 原子列上,CO途径不工作,电极未出现毒化现象
    ●甲酸能在1D Pt 原子列上氧化, 直接途径反应电流正比于台阶密度

    ●直接途径以此机理进行的可能性很小

     

    ●ChemPhysChem, 2007,8,380

    ●Phys. Chem. Chem. Phys., 2013, 15, 4625

    ●Phys. Chem. Chem. Phys., 2013, 15 , 4367

    ●Chinese Journal Of Chemical Physics, 2014, 16, 191, 2013, 26, 321, 2013, 26, 471

    ●J. Phys. Chem. C, 2014,118,6335

     


    甲酸电催化氧化机理研究

    Addr: 96 Jinzhai Rd Hefei Anhui P.R.China
    Laboratory of Spectrochemistry, Hefei National Laboratory for Physical Sciences at the Microscale
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